Förster resonance energy transfer, absorption and emission spectra in multichromophoric systems. II. Hybrid cumulant expansion
We develop a hybrid cumulant expansion method to account for the system-bath entanglement in the emission spectrum in the multi-chromophoric Förster transfer rate. In traditional perturbative treatments, the emission spectrum is usually expanded with respect to the system-bath coupling term in both...
Main Authors: | Ma, Jian, Moix, Jeremy, Cao, Jianshu |
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Other Authors: | Massachusetts Institute of Technology. Department of Chemistry |
Format: | Article |
Language: | en_US |
Published: |
American Institute of Physics (AIP)
2017
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Online Access: | http://hdl.handle.net/1721.1/110442 https://orcid.org/0000-0001-7616-7809 |
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