Surface Restructuring of Nickel Sulfide Generates Optimally Coordinated Active Sites for Oxygen Reduction Catalysis
The Ni₃S₂ bulk phase supports efficient oxygen reduction reaction (ORR) catalysis in pH neutral aqueous electrolytes. Here, we combine electrochemistry, surface spectroscopy, and high-resolution microscopy to show that Ni₃S₂ undergoes self-limiting oxidative surface restructuring under ORR conditio...
Main Authors: | Yan, Bing, Krishnamurthy, Dilip, Hendon, Christopher H, Deshpande, Siddharth, Surendranath, Yogesh, Viswanathan, Venkatasubramanian |
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Other Authors: | Massachusetts Institute of Technology. Department of Chemistry |
Format: | Article |
Language: | English |
Published: |
Elsevier BV
2020
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Online Access: | https://hdl.handle.net/1721.1/126863 |
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