Why Conventional Design Rules for C–H Activation Fail for Open-Shell Transition-Metal Catalysts
© 2020 American Chemical Society. The design of selective and active C−H activation catalysts for direct methane-to-methanol conversion is challenging. Bioinspired complexes that form high-valent metal−oxo intermediates capable of hydrogen abstraction and rebound hydroxylation are promising candidat...
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Format: | Article |
Language: | English |
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American Chemical Society (ACS)
2021
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Online Access: | https://hdl.handle.net/1721.1/134032 |