Theory of Layered-Oxide Cathode Degradation in Li-ion Batteries by Oxidation-Induced Cation Disorder
Disorder-driven degradation phenomena, such as structural phase transformations and surface reconstructions, can significantly reduce the lifetime of Li-ion batteries, especially those with nickel-rich layered-oxide cathodes. We develop a general free energy model for layered-oxide ion-intercalation...
Main Authors: | Zhuang, Debbie, Bazant, Martin Z |
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Other Authors: | Massachusetts Institute of Technology. Department of Chemical Engineering |
Format: | Article |
Language: | English |
Published: |
The Electrochemical Society
2024
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Online Access: | https://hdl.handle.net/1721.1/157531 |
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