Coherent two-exciton dynamics measured using two-quantum rephasing two-dimensional electronic spectroscopy

We use fifth-order two-dimensional electronic spectroscopy to measure coherent four-particle dynamics in a semiconductor nanostructure. By using optical polarization control in two-quantum measurements enabled by the COLBERT spectrometer, we separate coherent signals due to bound biexcitons and unbo...

Full description

Bibliographic Details
Main Authors: Turner, Daniel B., Wen, Patrick, Arias, Dylan H., Nelson, Keith Adam
Other Authors: Massachusetts Institute of Technology. Department of Chemistry
Format: Article
Language:en_US
Published: American Physical Society (APS) 2012
Online Access:http://hdl.handle.net/1721.1/68670
https://orcid.org/0000-0003-2358-6967
https://orcid.org/0000-0001-7804-5418