Hot Carrier-Assisted Intrinsic Photoresponse in Graphene

We report on the intrinsic optoelectronic response of high-quality dual-gated monolayer and bilayer graphene p-n junction devices. Local laser excitation (of wavelength 850 nanometers) at the p-n interface leads to striking six-fold photovoltage patterns as a function of bottom- and top-gate voltage...

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Main Authors: Gabor, Nathaniel M., Song, Justin Chien Wen, Ma, Qiong, Nair, Nityan L., Taychatanapat, Thiti, Levitov, Leonid, Jarillo-Herrero, Pablo, Watanabe, Kenji, Taniguchi, Takashi
Other Authors: Massachusetts Institute of Technology. Department of Physics
Format: Article
Language:en_US
Published: American Association for the Advancement of Science (AAAS) 2014
Online Access:http://hdl.handle.net/1721.1/88466
https://orcid.org/0000-0002-4268-731X
https://orcid.org/0000-0002-5103-6973
https://orcid.org/0000-0001-8217-8213
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author Gabor, Nathaniel M.
Song, Justin Chien Wen
Ma, Qiong
Nair, Nityan L.
Taychatanapat, Thiti
Levitov, Leonid
Jarillo-Herrero, Pablo
Watanabe, Kenji
Taniguchi, Takashi
author2 Massachusetts Institute of Technology. Department of Physics
author_facet Massachusetts Institute of Technology. Department of Physics
Gabor, Nathaniel M.
Song, Justin Chien Wen
Ma, Qiong
Nair, Nityan L.
Taychatanapat, Thiti
Levitov, Leonid
Jarillo-Herrero, Pablo
Watanabe, Kenji
Taniguchi, Takashi
author_sort Gabor, Nathaniel M.
collection MIT
description We report on the intrinsic optoelectronic response of high-quality dual-gated monolayer and bilayer graphene p-n junction devices. Local laser excitation (of wavelength 850 nanometers) at the p-n interface leads to striking six-fold photovoltage patterns as a function of bottom- and top-gate voltages. These patterns, together with the measured spatial and density dependence of the photoresponse, provide strong evidence that nonlocal hot carrier transport, rather than the photovoltaic effect, dominates the intrinsic photoresponse in graphene. This regime, which features a long-lived and spatially distributed hot carrier population, may offer a path to hot carrier–assisted thermoelectric technologies for efficient solar energy harvesting.
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spelling mit-1721.1/884662022-09-28T12:47:06Z Hot Carrier-Assisted Intrinsic Photoresponse in Graphene Gabor, Nathaniel M. Song, Justin Chien Wen Ma, Qiong Nair, Nityan L. Taychatanapat, Thiti Levitov, Leonid Jarillo-Herrero, Pablo Watanabe, Kenji Taniguchi, Takashi Massachusetts Institute of Technology. Department of Physics Gabor, Nathaniel M. Song, Justin Chien Wen Ma, Qiong Nair, Nityan L. Taychatanapat, Thiti Levitov, Leonid Jarillo-Herrero, Pablo We report on the intrinsic optoelectronic response of high-quality dual-gated monolayer and bilayer graphene p-n junction devices. Local laser excitation (of wavelength 850 nanometers) at the p-n interface leads to striking six-fold photovoltage patterns as a function of bottom- and top-gate voltages. These patterns, together with the measured spatial and density dependence of the photoresponse, provide strong evidence that nonlocal hot carrier transport, rather than the photovoltaic effect, dominates the intrinsic photoresponse in graphene. This regime, which features a long-lived and spatially distributed hot carrier population, may offer a path to hot carrier–assisted thermoelectric technologies for efficient solar energy harvesting. National Science Foundation (U.S.) (Early Career Award) David & Lucile Packard Foundation United States. Air Force Office of Scientific Research 2014-07-22T15:07:38Z 2014-07-22T15:07:38Z 2011-10 2011-07 Article http://purl.org/eprint/type/JournalArticle 0036-8075 1095-9203 http://hdl.handle.net/1721.1/88466 Gabor, N. M., J. C. W. Song, Q. Ma, N. L. Nair, T. Taychatanapat, K. Watanabe, T. Taniguchi, L. S. Levitov, and P. Jarillo-Herrero. “Hot Carrier-Assisted Intrinsic Photoresponse in Graphene.” Science 334, no. 6056 (November 4, 2011): 648–652. https://orcid.org/0000-0002-4268-731X https://orcid.org/0000-0002-5103-6973 https://orcid.org/0000-0001-8217-8213 en_US http://dx.doi.org/10.1126/science.1211384 Science Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use. application/pdf American Association for the Advancement of Science (AAAS) arXiv
spellingShingle Gabor, Nathaniel M.
Song, Justin Chien Wen
Ma, Qiong
Nair, Nityan L.
Taychatanapat, Thiti
Levitov, Leonid
Jarillo-Herrero, Pablo
Watanabe, Kenji
Taniguchi, Takashi
Hot Carrier-Assisted Intrinsic Photoresponse in Graphene
title Hot Carrier-Assisted Intrinsic Photoresponse in Graphene
title_full Hot Carrier-Assisted Intrinsic Photoresponse in Graphene
title_fullStr Hot Carrier-Assisted Intrinsic Photoresponse in Graphene
title_full_unstemmed Hot Carrier-Assisted Intrinsic Photoresponse in Graphene
title_short Hot Carrier-Assisted Intrinsic Photoresponse in Graphene
title_sort hot carrier assisted intrinsic photoresponse in graphene
url http://hdl.handle.net/1721.1/88466
https://orcid.org/0000-0002-4268-731X
https://orcid.org/0000-0002-5103-6973
https://orcid.org/0000-0001-8217-8213
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