Theory of femtosecond coherent double-pump single-molecule spectroscopy : application to light harvesting complexes
We develop a first principles theoretical description of femtosecond double-pump single-molecule signals of molecular aggregates. We incorporate all singly-excited electronic states and vibrational modes with significant electron-vibrational coupling into a system Hamiltonian and treat the ensuing s...
| Main Authors: | , , , |
|---|---|
| Other Authors: | |
| Format: | Journal Article |
| Language: | English |
| Published: |
2015
|
| Subjects: | |
| Online Access: | https://hdl.handle.net/10356/107369 http://hdl.handle.net/10220/25478 |