Spin versus boson baths in nonlinear spectroscopy
The third-order optical response function of a chromophore coupled to a bath consisting of noninteracting two-level systems (TLSs) undergoing stochastic jumps is calculated. The results can be applied to a broad class of nonlinear optical techniques in single-molecule spectroscopy and bulk measureme...
Huvudupphovsmän: | , , |
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Materialtyp: | Journal Article |
Språk: | English |
Publicerad: |
2011
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Länkar: | https://hdl.handle.net/10356/93955 http://hdl.handle.net/10220/7419 |