Spin versus boson baths in nonlinear spectroscopy
The third-order optical response function of a chromophore coupled to a bath consisting of noninteracting two-level systems (TLSs) undergoing stochastic jumps is calculated. The results can be applied to a broad class of nonlinear optical techniques in single-molecule spectroscopy and bulk measureme...
| Main Authors: | , , |
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| Other Authors: | |
| Format: | Journal Article |
| Language: | English |
| Published: |
2011
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| Subjects: | |
| Online Access: | https://hdl.handle.net/10356/93955 http://hdl.handle.net/10220/7419 |