Extremely well isolated two-dimensional spin-1/2 antiferromagnetic Heisenberg layers with a small exchange coupling in the molecular-based magnet CuPOF

We report on a comprehensive characterization of the newly synthesized Cu2+-based molecular magnet [Cu(pz)2(2-HOpy)2](PF6)2 (CuPOF), where pz=C4H4N2 and 2-HOpy=C5H4NHO. From a comparison of theoretical modeling to results of bulk magnetometry, specific heat, μ+SR, ESR, and NMR spectroscopy, this mat...

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Bibliographic Details
Main Authors: Opherden, D, Nizar, N, Richardson, K, Monroe, JC, Turnbull, MM, Polson, M, Vela, S, Blackmore, WJA, Goddard, PA, Singleton, J, Choi, ES, Xiao, F, Williams, RC, Lancaster, T, Pratt, FL, Blundell, SJ, Skourski, Y, Uhlarz, M, Ponomaryov, AN, Zvyagin, SA, Wosnitza, J, Baenitz, M, Heinmaa, I, Stern, R, Kuhne, H, Landee, CP
Format: Journal article
Language:English
Published: American Physical Society 2020