Singlet triplet-pair production and possible singlet-fission in carotenoids
Internal conversion from the photoexcited state to a correlated singlet triplet-pair state is believed to be the precursor of singlet fission in carotenoids. We present numerical simulations of this process using a π-electron model that fully accounts for electron–electron interactions and electron–...
Главные авторы: | Manawadu, D, Valentine, D, Marcus, M, Barford, W |
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Формат: | Journal article |
Язык: | English |
Опубликовано: |
American Chemical Society
2022
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