Understanding strong two-photon absorption in pi-conjugated porphyrin dimers via double-resonance enhancement in a three-level model.
We present the two-photon absorption (2PA) spectra of a series of conjugated porphyrin dimers and show that they possess extremely large intrinsic (femtosecond) peak 2PA cross sections, up to sigma2 = 1 x 104 GM in the near-IR region; these are among the highest values measured for any organic molec...
Main Authors: | , , , , , , |
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Format: | Journal article |
Language: | English |
Published: |
2004
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