Theory of singlet fission in carotenoid dimers
We develop a theory of singlet fission in carotenoid dimers. Following photoexcitation of the “bright” state (i.e., a singlet electron–hole pair) in a single carotenoid, the first step in the singlet fission process is ultrafast intramolecular conversion into the highly correlated “dark” (or 2Ag) st...
| Main Authors: | , |
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| Format: | Journal article |
| Language: | English |
| Published: |
American Institute of Physics
2023
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