Magnetic phase transitions in the two-dimensional frustrated quantum antiferromagnet Cs2CuCl4

We report magnetization and specific heat measurements in the 2D frustrated spin-1/2 Heisenberg antiferromagnet Cs2CuCl4 at temperatures down to 0.05 K and high magnetic fields up to 11.5 T applied along a, b and c-axes. The low-field susceptibility chi (T) M/B shows a broad maximum around 2.8 K cha...

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Main Authors: Tokiwa, Y, Radu, T, Coldea, R, Wilhelm, H, Tylczynski, Z, Steglich, F
Format: Journal article
Language:English
Published: 2006
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author Tokiwa, Y
Radu, T
Coldea, R
Wilhelm, H
Tylczynski, Z
Steglich, F
author_facet Tokiwa, Y
Radu, T
Coldea, R
Wilhelm, H
Tylczynski, Z
Steglich, F
author_sort Tokiwa, Y
collection OXFORD
description We report magnetization and specific heat measurements in the 2D frustrated spin-1/2 Heisenberg antiferromagnet Cs2CuCl4 at temperatures down to 0.05 K and high magnetic fields up to 11.5 T applied along a, b and c-axes. The low-field susceptibility chi (T) M/B shows a broad maximum around 2.8 K characteristic of short-range antiferromagnetic correlations and the overall temperature dependence is well described by high temperature series expansion calculations for the partially frustrated triangular lattice with J=4.46 K and J'/J=1/3. At much lower temperatures (< 0.4 K) and in in-plane field (along b and c-axes) several new intermediate-field ordered phases are observed in-between the low-field incommensurate spiral and the high-field saturated ferromagnetic state. The ground state energy extracted from the magnetization curve shows strong zero-point quantum fluctuations in the ground state at low and intermediate fields.
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spelling oxford-uuid:cfd86bf9-2db0-49f8-b811-1ed8325f8fb22022-03-27T07:45:39ZMagnetic phase transitions in the two-dimensional frustrated quantum antiferromagnet Cs2CuCl4Journal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:cfd86bf9-2db0-49f8-b811-1ed8325f8fb2EnglishSymplectic Elements at Oxford2006Tokiwa, YRadu, TColdea, RWilhelm, HTylczynski, ZSteglich, FWe report magnetization and specific heat measurements in the 2D frustrated spin-1/2 Heisenberg antiferromagnet Cs2CuCl4 at temperatures down to 0.05 K and high magnetic fields up to 11.5 T applied along a, b and c-axes. The low-field susceptibility chi (T) M/B shows a broad maximum around 2.8 K characteristic of short-range antiferromagnetic correlations and the overall temperature dependence is well described by high temperature series expansion calculations for the partially frustrated triangular lattice with J=4.46 K and J'/J=1/3. At much lower temperatures (< 0.4 K) and in in-plane field (along b and c-axes) several new intermediate-field ordered phases are observed in-between the low-field incommensurate spiral and the high-field saturated ferromagnetic state. The ground state energy extracted from the magnetization curve shows strong zero-point quantum fluctuations in the ground state at low and intermediate fields.
spellingShingle Tokiwa, Y
Radu, T
Coldea, R
Wilhelm, H
Tylczynski, Z
Steglich, F
Magnetic phase transitions in the two-dimensional frustrated quantum antiferromagnet Cs2CuCl4
title Magnetic phase transitions in the two-dimensional frustrated quantum antiferromagnet Cs2CuCl4
title_full Magnetic phase transitions in the two-dimensional frustrated quantum antiferromagnet Cs2CuCl4
title_fullStr Magnetic phase transitions in the two-dimensional frustrated quantum antiferromagnet Cs2CuCl4
title_full_unstemmed Magnetic phase transitions in the two-dimensional frustrated quantum antiferromagnet Cs2CuCl4
title_short Magnetic phase transitions in the two-dimensional frustrated quantum antiferromagnet Cs2CuCl4
title_sort magnetic phase transitions in the two dimensional frustrated quantum antiferromagnet cs2cucl4
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